Coherent diffractive imaging of graphite nanoparticles using a tabletop EUV source

Literature Information

Publication Date 2017-10-23
DOI 10.1039/C7CP03145A
Impact Factor 3.676
Authors

Ilya Strashnov, Eric Whittaker, Xiang Li Zhong


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Abstract

Structural information of nanostructures plays a key role in synthesis of novel nano-sized materials for promising applications such as high-performance nanoelectronics and nanophotonics. In this study, we apply for the first time the state-of-the-art coherent diffractive imaging method to characterize the structure of graphite nanoparticles. A sample with nanographites on a Si3N4 support was exposed to 30 nm radiation from a tabletop laser-driven high-order harmonic generation extreme ultraviolet (EUV) source. From the measured far-field diffraction pattern, we were able to reconstruct the distribution of the graphite nanoparticles with a spatial resolution of ∼330 nm using the standard iterative phase retrieval algorithms. A closer look at the reconstructed images reveals possible absorption effects of graphite nanoparticles. This experiment demonstrates the first step towards wide-field and high-resolution imaging of nuclear materials using the newly established lab-scale EUV source. Having such a source opens the door to performing investigations of nuclear graphite and other radioactive material in the lab, thus avoiding the need to transport samples to external facilities.

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Source Journal

Physical Chemistry Chemical Physics

Physical Chemistry Chemical Physics
CiteScore: 5.5
Self-citation Rate: 10.3%
Articles per Year: 3036

Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions. The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.

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