Facile one-pot/one-step synthesis of heterotelechelic N-acylated poly(aminoester) macromonomers for carboxylic acid decorated comb polymers
Literature Information
Publication Date
2016-10-19
DOI
10.1039/C6PY01553K
Impact Factor
5.582
Authors
Patrick A. J. M. de Jongh, Mechelle R. Bennett, Greg S. Sulley
View Original
Abstract
Optimised monomer feed ratios in the spontaneous zwitterionic copolymerisation (SZWIP) of 2-oxazolines and acrylic acid enable the one-step synthesis of heterotelechelic α-acrylate, ω-carboxylic acid N-acylated poly(aminoester) macromonomers. Subsequent redox-initiated RAFT polymerisation at ambient temperature leads to comb polymers containing quantitative terminal side chain carboxylic acids, which allow efficient ‘grafting-onto’ using conventional peptide coupling strategies.
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Source Journal
Polymer Chemistry
CiteScore:
8.6
Self-citation Rate:
7.3%
Articles per Year:
457
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