Oxygen tolerant, photoinduced controlled radical polymerization approach for the synthesis of giant amphiphiles
Literature Information
Publication Date
2021-03-18
DOI
10.1039/D0PY01608J
Impact Factor
5.582
Authors
Alexis Theodorou, Petros Mandriotis, Athina Anastasaki, Kelly Velonia
View Original
Abstract
Amphiphilic protein–polymer conjugates form hybrid nanostructures with a broad range of potential applications. Herein, we expand the scope of amphiphilic protein–polymer bioconjugates via an oxygen tolerant, photoinduced RDRP method. A range of hydrophobic acrylic, methacrylic and acrylamide-based monomers are comprehensively screened to identify optimum reaction conditions that lead to quantitative biomacroinitiator consumption. By judiciously varying a number of components (e.g. monomer loading, catalyst concentration, pH, co-solvent, salt content), well-defined protein–polymer conjugates bearing different polymer moieties were obtained and their intrinsic properties were expressed through both their self-assembled architectures and esterase-like catalytic activity.
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Source Journal
Polymer Chemistry
CiteScore:
8.6
Self-citation Rate:
7.3%
Articles per Year:
457
Polymer Chemistry welcomes submissions in all areas of polymer science that have a strong focus on macromolecular chemistry. Manuscripts may cover a broad range of fields, yet no direct application focus is required.
Recommended Compounds
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![tert-butyl 8-benzyl-2,8-diazaspiro[4.5]decane-2-carboxylate structure](https://static.chemtradehub.com/structs/336/336191-16-3-bb55.webp "tert-butyl 8-benzyl-2,8-diazaspiro[4.5]decane-2-carboxylate structure")
tert-butyl 8-benzyl-2,8-diazaspiro[4.5]decane-2-carboxylate
CAS Number:
336191-16-3
Molecular Formula:
C20H30N2O2
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