Iminyl radical-promoted imino sulfonylation, imino cyanogenation and imino thiocyanation of γ,δ-unsaturated oxime esters: synthesis of versatile functionalized pyrrolines
Literature Information
Publication Date
2019-05-06
DOI
10.1039/C9QO00421A
Impact Factor
5.281
Authors
Yuebo Wang, Jie Ding, Jinghui Zhao, Wan Sun, Chang Lian, Chen Chen, Bolin Zhu
View Original
Abstract
An efficient approach for the cascade radical cyclization/functionalization of γ,δ-unsaturated oxime esters was developed, which introduced useful functional groups (–SO2R, –CN, –SCN) into pyrrolines. Control experiments were conducted and a mechanism involving iminyl radical intermediates, which was initiated by Cu(I) species, was proposed.
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Source Journal
Organic Chemistry Frontiers
CiteScore:
7.8
Self-citation Rate:
8.7%
Articles per Year:
724
Organic Chemistry Frontiers publishes high-quality research from across organic chemistry. Emphases are placed on studies that make significant contributions to the field of organic chemistry by reporting either new or significantly improved protocols or methodologies. Topics include, but are not limited to the following: Organic synthesis Development of synthetic methodologies Catalysis Natural products Functional organic materials Supramolecular and macromolecular chemistry Physical and computational organic chemistry
Recommended Compounds
Oxalic acid compound with cyclohexylsulfamothioic O-acid (11)
CAS Number:
31895-22-4
Molecular Formula:
C7H13NO4S3
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2,9-Dichloro-5,12-dihydroquinolino[2,3-b]acridine-7,14-dione
CAS Number:
3089-17-6
Molecular Formula:
C20H10Cl2N2O2
![N-[(E)-Phenylmethylene]benzenesulfonamide structure](https://static.chemtradehub.com/structs/139/13909-34-7-8167.webp "N-[(E)-Phenylmethylene]benzenesulfonamide structure")
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