A well-defined nitro-functionalized aromatic framework (NO2-PAF-1) with high CO2 adsorption: synthesis via the copper-mediated Ullmann homo-coupling polymerization of a nitro-containing monomer
Literature Information
Publication Date
2015-11-24
DOI
10.1039/C5PY01682G
Impact Factor
5.582
Authors
Ze-Huan Hei, Mu-Hua Huang, Yunjun Luo, Yingxiong Wang
View Original
Abstract
A well-defined nitro group functionalized porous aromatic framework (NO2-PAF-1) was synthesized via a bottom-up strategy using a copper-mediated Ullmann reaction. The synthetic route is cost-efficient and robust for large scale preparation. The Brunauer–Emmett–Teller (BET) specific surface area of the obtained NO2-PAF-1 is up to 610 cm2 g−1 with micro/mesoporosity. Its CO2 uptake was measured to be higher than that of PAF-1 due to the strong interaction between the nitro groups and CO2 molecules, proven by the enhanced isosteric heat of CO2 adsorption (38.4 kJ mol−1).
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Source Journal
Polymer Chemistry
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8.6
Self-citation Rate:
7.3%
Articles per Year:
457
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C11H12N2OS
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(1R,2R)-2-Methylcyclohexanamine hydrochloride (1:1)
CAS Number:
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Molecular Formula:
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