Synthesis of a controlled three-faced PAMAM particle

Literature Information

Publication Date 2011-07-14
DOI 10.1039/C1PY00146A
Impact Factor 5.582
Authors

Mathieu Arseneault, Philippe Dufour, Isabelle Levesque, Jean-François Morin


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Abstract

We report the synthetic proof-of-concept for a three-faced particle based on a PAMAM dendrimer in which each face bears a different labile protecting group. This new strategy yields a controlled, well-defined and monodisperse dendrimer. To achieve this, a tri-orthogonal strategy was employed through Sonogashira coupling and Cu(I)-catalyzed Huisgen [2 + 3] dipolar cycloaddition (“click” chemistry). The afforded dendrimer is well suited for further development in a variety of fields as each branch can be addressed individually for functionalization.

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