CO2 hydrogenation to olefins in a microwave-thermal hybrid heating reactor

Literature Information

Publication Date 2023-12-26
DOI 10.1039/D3RE00636K
Impact Factor 4.239
Authors

Sonit Balyan, Kshitij Tewari, Brandon Robinson, Changle Jiang, Yuxin Wang, Jianli Hu


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Abstract

In this study, an approach based on microwave-enhanced CO2 hydrogenation to olefins was carried out in a two-zone hybrid heating reactor system at moderate pressures of 20–140 psig. Methanol synthesis was conducted in a microwave heated zone over a stable Cu/ZnO/Al2O3 catalyst and the methanol conversion to olefins was conducted in a conventional thermally heated zone over SAPO-34 zeolite. This work demonstrates the potential of microwave-driven catalytic technology to decarbonize greenhouse gases into valuable chemicals utilizing green hydrogen under mild conditions.

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Source Journal

Reaction Chemistry & Engineering

Reaction Chemistry & Engineering
CiteScore: 0
Self-citation Rate: 8.8%
Articles per Year: 284

Reaction Chemistry & Engineering is an interdisciplinary journal reporting cutting-edge research focused on enhancing the understanding and efficiency of reactions. Reaction engineering leverages the interface where fundamental molecular chemistry meets chemical engineering and technology. Challenges in chemistry can be overcome by the application of new technologies, while engineers may find improved solutions for process development from the latest developments in reaction chemistry. Reaction Chemistry & Engineering is a unique forum for researchers whose interests span the broad areas of chemical engineering and chemical sciences to come together in solving problems of importance to wider society. All papers should be written to be approachable by readers across the engineering and chemical sciences. Papers that consider multiple scales, from the laboratory up to and including plant scale, are particularly encouraged.

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