How to go beyond C1 products with electrochemical reduction of CO2

Literature Information

Publication Date 2021-10-20
DOI 10.1039/D1SE00861G
Impact Factor 6.367
Authors

Hao Zhang, Hang Xiang, Shahid Rasul, Alberto Roldan, Rebecca Taylor, Yujie Feng, Liam Banerji, Alexander Cowan, Jin Xuan


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Abstract

The electrochemical reduction of CO2 to produce fuels and value-added organic chemicals is of great potential, providing a mechanism to convert and store renewable energy within a carbon-neutral energy circle. Currently the majority of studies report C1 products such as carbon monoxide and formate as the major CO2 reduction products. A particularly challenging goal within CO2 electrochemical reduction is the pursuit of multi-carbon (C2+) products which have been proposed to enable a more economically viable value chain. This review summaries recent development across electro-, photoelectro- and bioelectro-catalyst developments. It also explores the role of device design and operating conditions in enabling C–C bond generation.

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