Highly chemoselective hydrogenation of cyclic imides to ω-hydroxylactams or ω-hydroxyamides catalyzed by iridium catalysts
Literature Information
Publication Date
2021-09-30
DOI
10.1039/D1QO01100F
Impact Factor
5.281
Authors
Jiang Wang, Xumu Zhang, Runtong Zhang, Baode Ma
View Original
Abstract
Several novel ferrocene-based PNN ligands were prepared, which were found to be highly effective catalysts (TON up to 50 000) for the homogeneous hydrogenation of cyclic imides with iridium. The hydrogenation mode (type I: ring opening/type II: non-ring opening) could be finely tuned by tiny changes in the ligands. Using this straightforward strategy, a plethora of ω-hydroxylactams and ω-hydroxyamides with different functional groups were obtained in high yield.
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Source Journal
Organic Chemistry Frontiers
CiteScore:
7.8
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8.7%
Articles per Year:
724
Organic Chemistry Frontiers publishes high-quality research from across organic chemistry. Emphases are placed on studies that make significant contributions to the field of organic chemistry by reporting either new or significantly improved protocols or methodologies. Topics include, but are not limited to the following: Organic synthesis Development of synthetic methodologies Catalysis Natural products Functional organic materials Supramolecular and macromolecular chemistry Physical and computational organic chemistry
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Molecular Formula:
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