Electronic transport properties and magnetoresistance in the Fe3O4/SiO2/p-Si heterostructure with an in-plane current geometry

Literature Information

Publication Date 2019-03-06
DOI 10.1039/C9CP00033J
Impact Factor 3.676
Authors

Xiang Liu, Wenbo Mi


View Original

Abstract

In traditional electronic devices, the electronic charge is manipulated to realize different functions. The fascinating control of electronic spin in conventional semiconductors increases the probability of occurrence of spin-dependent transport properties. Herein, the injection of electronic spin into a Si wafer with in-plane geometry was achieved by Fe3O4, which acted as a spin injector. At high temperatures, the resistivity of Fe3O4 is far less than that of a p-Si wafer. Moreover, above 190 K, the current–voltage (I–V) characteristic and magnetoresistance (MR) of the proposed heterostructure are dominated by the intrinsic properties of a polycrystalline Fe3O4 film, and the in-plane current flows in the Fe3O4 layer. Due to the increased resistivity of Fe3O4 at low temperatures, the in-plane conductive channel gradually switches from Fe3O4 to Si. The spin injection from Fe3O4 results in a spin-polarized space charge region in p-Si. The heterostructure shows an MR of up to −76.1% at 90 K due to the spin-dependent transport of electrons in p-Si. With a further decrease in temperature, the I–V characteristic of the heterostructure shows negative differential resistance below 80 K due to band bending at the Fe3O4/SiO2/p-Si interface.

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Physical Chemistry Chemical Physics

Physical Chemistry Chemical Physics
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Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions. The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.

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