Electronic effects of ligand substitution on metal–organic framework photocatalysts: the case study of UiO-66

Literature Information

Publication Date 2014-11-03
DOI 10.1039/C4CP04162C
Impact Factor 3.676
Authors

Lijuan Shen, Ruowen Liang, Mingbu Luo, Fenfen Jing, Ling Wu


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Abstract

UiO-66-X (X = H, NH2, NO2, Br) have been successfully synthesized and tested for their photocatalytic activity in water treatment. Results show that electronic effect of the ligand substituents greatly affects the photocatalytic activity of UiO-66. The rates obtained by different substituents are linearly correlated with their Hammett coefficients.

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Physical Chemistry Chemical Physics

Physical Chemistry Chemical Physics
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Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions. The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.

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