From degeneration to damping of electrochemical oscillation induced by temperature controlling of heat-compensation type

Literature Information

Publication Date 2002-02-19
DOI 10.1039/B108572G
Impact Factor 3.676
Authors

Jinglei Lei, Jiuli Luo


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Abstract

Instead of the passivation of the electrode surface, another approach leading to the nonsustaining character of electrochemical oscillation induced by temperature control of heat-compensation type is suggested in this paper. As an illustration the thermokinetic behavior of the anodic dissolution of copper in acidic chloride solution influenced by both the chemical reaction–heat conduction coupling and the temperature undulation in the controlling error range has been analyzed quantitatively. It turned out that this kind of temperature fluctuation will lead to limit cycle type degeneration of the sustained electrode chemical oscillation. As a result, two kinds of evolutionary perspectives, both the quasi-periodic oscillation and the damping oscillation, are expected.

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Physical Chemistry Chemical Physics

Physical Chemistry Chemical Physics
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Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions. The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.

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