Nuclear dynamics in quantum clusters

Literature Information

Publication Date 2001-05-18
DOI 10.1039/B100550M
Impact Factor 3.676
Authors

Andreas Heidenreich, Isidore Last, Uzi Even, Joshua Jortner


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Abstract

We address recent developments in the exploration of quantum nuclear dynamics in large, finite, low-temperature systems, focusing on Bose–Einstein condensates (T≃100 nK), optical molasses (T≃10–100 μK) and aromatic molecule·Hen clusters (T = 0.4 K). The expansion of optical molasses bears a close analogy to the nuclear dynamics of Coulomb explosion of multicharged clusters. Spectroscopy of electronic–vibrational excitations of anthracene·Hen clusters manifests large nuclear quantum effects, nonrigidity, large scale confinement and permutational symmetry effects. Perspectives for the novel research area of nuclear dynamics of ultracold finite systems are advanced.

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Physical Chemistry Chemical Physics

Physical Chemistry Chemical Physics
CiteScore: 5.5
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Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions. The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.

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