Homogeneous freezing nucleation rates and crystallization dynamics of single levitated sulfuric acid solution droplets
Literature Information
Hermann Vortisch, Benedikt Krämer, Inez Weidinger, Ludger Wöste, Thomas Leisner, Martin Schwell, Helmut Baumgärtel, Eckart Rühl
Supercooled sulfuric acid solution droplets are a major constituent of the stratospheric background aerosol. We report the rate of homogeneous freezing and the crystallization dynamics of single levitated sulfuric acid solution droplets with 0 to 57.6 wt.% H2SO4. The energy of formation of the critical nucleus and the self-diffusion activation energy are deduced from the experiments as a function of temperature and concentration. The results are compared to both theoretical and experimental work of other groups.
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