Nanoscale detection of metal-labeled copolymers in patchy polymersomes

Literature Information

Publication Date 2015-01-05
DOI 10.1039/C4PY01508H
Impact Factor 5.582
Authors

Jeppe Madsen, Efrosyni Themistou, Steven P. Armes


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Abstract

We report the synthesis of polymersome-forming block copolymers using two different synthetic routes based on Atom Transfer Radical Polymerization (ATRP) and Reversible Addition Fragmentation chain Transfer (RAFT) polymerization, respectively. Functionalization with 1,4,7,10-tetraazacyclododecane-1,4,7,10-tetraacetic acid (DOTA) allowed the block copolymer chains to be labelled with electron-dense metal ions (e.g. indium). The resulting metal-conjugated copolymers can be visualized by transmission electron microscopy with single chain resolution, hence enabling the study of polymer/polymer immiscibility and phase separation on the nano-scale.

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Polymer Chemistry

Polymer Chemistry
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