Ultrafast dynamics of the 11Bu-state of 1,3-butadiene after excitation at 204 nm

Literature Information

Publication Date 2001-07-02
DOI 10.1039/B104013H
Impact Factor 3.676
Authors

Frank Assenmacher, Michael Gutmann, Georg Hohlneicher, Volker Stert, Wolfgang Radloff


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Abstract

The ultrafast dynamics of the 11Bu state of 1,3-butadiene was investigated in real time in a femtosecond pump–probe experiment utilizing the RE2PI scheme. A lifetime of 35 ± 10 fs was found for the 11Bu state of the jet-cooled molecule.

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Physical Chemistry Chemical Physics

Physical Chemistry Chemical Physics
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Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions. The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.

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