A rational guide to improve the activity of a hydrogen-evolving polymeric carbon nitride photocatalyst
Literature Information
Publication Date
2023-11-21
DOI
10.1039/D3SE00996C
Impact Factor
6.367
Authors
Tomoharu Maeda, Chomponoot Suppaso, Shunta Nishioka, Yoshinobu Kamakura, Shuhei Yasuda, Toshiyuki Yokoi
View Original
Abstract
Photocatalytic H2 evolution using Pt-loaded mesoporous polymeric carbon nitride (meso-PCN) was studied with respect to light intensity and the hydrogen窶電euterium isotope effect, in combination with photoelectrochemical measurements. Although the photocatalytic activity was mainly limited by charge recombination in the meso-PCN, improving the oxidation reaction by photogenerated holes was critical for enhancing the H2-evolution activity. The finding of this work will be a useful guide to achieve non-sacrificial overall water splitting by PCN photocatalysts.
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