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Red-shifted activity-based sensors for ethylene via direct conjugation of fluorophore to metal–carbene
Literature Information
Publication Date
2023-09-25
DOI
10.1039/D3CB00079F
Impact Factor
0
Authors
Nicholas J. Dacon, Nathan B. Wu, Brian W. Michel
View Original
Abstract
A number of Activity-Based Sensors (ABS) for relatively unreactive small molecules, such as ethylene, necessitates a transition metal for reaction under ambient conditions. Olefin metathesis has emerged as one of the primary strategies to achieve ethylene detection, and other transition metals are used for similarly challenging-to-detect analytes. However, limited studies exist investigating how fluorophore-metal attachment impacts photophysical properties of such ABS. Two new probes were prepared with the chelating benzlidene Ru–ligand directly conjugated to a BODIPY fluorophore and the photophysical properties of the new conjugated ABS were evaluated.
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